鎽樿锛氶毃钁楀畨鍏ㄨ姹傜殑鎻愰珮,娑叉皑浣滅偤鐕冪叅闆诲粻鑴閭勫師鍔戝皣閫愭琚翱绱犲彇浠�銆傛弿杩板翱绱犳按瑙ｈ垏灏跨礌?z茅)宄らェ澶筭(sh霉),骞朵互2脳1000MW鐕冪叅鐧�(f膩)闆绘(j墨)绲勬敼閫犻爡(xi脿ng)鐩偤渚�,寰炴妧琛�(sh霉)鎬ц垏缍�(j墨ng)婵�(j矛)鎬ц搴︽瘮杓冧簡灏跨礌姘磋В鑸囧翱绱�?z茅)宄ゅい銇殥?br />
鐕冪叅闆诲粻鑴鐢ㄩ倓鍘熷姂涓€鑸湁娑叉皑銆佹皑姘村拰灏跨礌銆傛恫姘ㄦ柟妗堝湪鎶曡硣鑸囬亱(y霉n)琛屾垚鏈笂鍏锋湁鏄庨’鍎�(y艒u)鍕�锛� 鍦嬪収(n猫i)澶ч儴鍒嗙噧鐓ら浕寤犻兘閬告搰娑叉皑浣滅偤閭勫師鍔�銆傞浕寤犳恫姘ㄥ劜閲忎竴鑸秴閬�10t锛屾牴鎿�(j霉)銆婂嵄闅�(xi菐n)鍖栧(xu茅)鍝侀噸澶у嵄闅�(xi菐n)婧愯鲸璀樸€�(GB/18218-2009) 鐨勭浉闂�(gu膩n)瑕�(gu墨)瀹氾紝妲�(g貌u)鎴愰噸澶у嵄闅�(xi菐n)婧�銆傚湅瀹跺皪瀹夊叏閬�(y霉n)琛岀殑瑕佹眰鏃ョ泭鍤�(y谩n)鏍�锛岄毃钁椼€婇棞(gu膩n)浜庡姞寮�(qi谩ng)鐕冪叅姗�(j墨)绲勮劔纭劔纭濆畨鍏ㄧ洠(ji膩n)鐫ｇ鐞嗙殑閫氱煡銆�( 鍦嬭兘瀹夊叏[2013]296 铏�)銆併€婄噧鐓ょ櫦(f膩)闆诲粻娑叉皑缃愬崁(q奴)瀹夊叏绠＄悊瑕�(gu墨)瀹氥€嬬瓑鏂囦欢鐨勫嚭鑷�锛� 鐕冪叅闆诲粻灏囪劔纭濋倓鍘熷姂鐢辨恫姘ㄥ崌绱氱偤灏跨礌鏄嫝鍦ㄥ繀琛岀殑銆�

1 灏跨礌鍒舵皑宸ヨ棟绨′粙

灏跨礌鍒舵皑宸ヨ棟鐨勪富瑕佸彲鍒嗙偤灏跨礌婧舵恫鍒跺倷鑸囧瓨鍎蹭互鍙婂翱绱犲垎瑙ｅ埗姘ㄥ叐閮ㄥ垎銆傛牴鎿�(j霉)灏跨礌鍒嗚В鍒舵皑宸ヨ棟鐨勪笉鍚岋紝灏跨礌鍒舵皑宸ヨ棟鍒嗙偤灏跨礌姘磋В宸ヨ棟鍜屽翱绱�?z茅)宄ゅい銇殥?br />
(1)灏跨礌姘磋В宸ヨ棟銆傚翱绱犳按瑙ｆ妧琛�(sh霉)鐢ㄤ簬鑴閭勫師鍔戝埗鍌欏湪鍦嬪閸嬬垚鐓欐埃鑴宸ョ▼涓緱鍒版噳(y墨ng)鐢ㄥ凡鏈夎純闀锋檪(sh铆)闁�銆傚翱绱犳按瑙ｅ弽鎳�(y墨ng)鏄翱绱犵敓鐢�(ch菐n)閬庣▼鐨勯€嗗弽鎳�(y墨ng)锛屽叾鍙嶆噳(y墨ng)鍙互瑾�(r猫n)鐐虹敱2姝ョ祫鎴愶細

NH2CONH2+H2O=NH2COONH4-15.5kJ/mol

NH2COONH4=2HN3+CO2+177kJ/mol

绗�1 姝ュ弽鎳�(y墨ng)鐐哄翱绱犺垏姘寸敓鎴愭皑鍩虹敳閰歌兒楣�锛� 瑭查亷绋嬬偤寰斁鐔卞弽鎳�(y墨ng)锛屽弽鎳�(y墨ng)閬庣▼闈炲父绶╂參;绗�2 姝ュ弽鎳�(y墨ng)鐐哄挤(qi谩ng)鍚哥啽鍙嶆噳(y墨ng)锛屾皑鍩虹敳閰歌兒杩呴€熷垎瑙ｇ敓鎴怤H3鍜孋O2锛屽弽鎳�(y墨ng)閬庣▼闈炲父杩呴€�銆�

灏嶄簬姘撮亷鍓╃殑灏跨礌婧舵恫锛岄亷閲忔按鐨勫瓨鍦ㄥ彲鍔犲揩鍙嶆噳(y墨ng)閫熷害銆�

鍦ㄦ湁閬庨噺姘村弮鑸囩殑鎯呮硜涓�锛屽翱绱犳按瑙ｇ附鐨勫寲瀛�(xu茅)鍙嶆噳(y墨ng)寮忕偤锛�

NH2CONH2+xH2O=2NH3鈫�+CO2鈫�+(x-1)H2O+161.5kJ/mol

灏跨礌婧舵恫鍦�130锝�160鈩冨弽鎳�(y墨ng)婧害鍜�0.4锝�0.6MPa 鍙嶆噳(y墨ng)澹撳姏姊濅欢涓嬬櫦(f膩)鐢熸按瑙ｅ弽鎳�(y墨ng)锛岀敘(ch菐n)鐢烴H3銆丠2O 鍜孋O2鐨勬贩鍚堟埃楂�銆傛按瑙ｅ弽鎳�(y墨ng)鍣ㄥ収(n猫i)閮ㄧ祼(ji茅)妲�(g貌u)濡傚湒1鎵€绀�锛� 姘磋В鍙嶆噳(y墨ng)鍣ㄥ収(n猫i)灏跨礌婧舵恫瀹圭⿳鐜囦竴鑸帶鍒跺湪70%浠ヤ笅锛屼笂閮ㄧ┖闁撲綔鐐烘按瑙ｆ埃鐨勭珐瀛樼┖闁�锛屼竴鑸爯(y霉)鐣�3锝�5min 鐨勯渶姘ㄩ噺锛屼互鎻愰珮鍏跺皪閸嬬垚璨�(f霉)鑽风殑闊挎噳(y墨ng)鎬с€�


鍌寲姘磋В鏄湪鏅€氭按瑙ｇ殑鍩虹(ch菙)涓�锛� 鍦ㄥ垵娆℃姇閬�(y霉n)鏅�(sh铆)娣诲姞涓€绋７閰搁姩楣介鍌寲鍔戝埌姘磋В鍙嶆噳(y墨ng)鍣ㄥ収(n猫i)锛� 閫氶亷鍌寲鍔戠殑鍌寲浣滅敤锛屼娇灏跨礌鍦ㄦ韩搴�135锝�160鈩�銆佸鍔�0.4锝�0.9MPa 涓嬮€�(j矛n)琛屽揩閫熸按瑙ｅ弽鎳�(y墨ng)锛岄熆鎳�(y墨ng)鏅�(sh铆)闁撳彲閬�(d谩)鍒�1min 浠ュ収(n猫i)銆�

鍌寲姘磋В娉曞叾鍖栧(xu茅)鍙嶆噳(y墨ng)寮忕偤锛�

CO(NH2)2+2NH4H2PO4+H2O鈫�2(NH4)2HPO4+CO2鈫�

2(NH4)2HPO4鈫�2NH3鈫�+2NH4H2PO4

缍滃悎鍙嶆噳(y墨ng)锛欳O(NH2)2+H2O鈫扖O2鈫�+2NH3鈫�

灏跨礌鍌寲姘磋В鏄湪鏅€氭按瑙ｇ殑鍩虹(ch菙)涓婏紝 鍦ㄥ翱绱犳按瑙ｉ亷绋嬩腑娣诲姞纾烽吀楣戒綔鐐哄偓鍖栧姂鏀硅畩鍙嶆噳(y墨ng)璺緫锛屽姞蹇弽鎳�(y墨ng)閫熺巼锛屾彁闊挎噳(y墨ng)閫熺巼銆�

(2) 灏跨礌?z茅)宄ゅい銇�?銆傜啽瑙ｆ妧琛�(sh霉)鏄埄鐢ㄧ啽绌烘埃浣滅偤鐔辨簮鍦�450锝�600鈩冨揩閫熷垎瑙�40%-50%鐨勫翱绱犳憾娑�銆傚弽鎳�(y墨ng)鏂圭▼寮忕偤锛�

CO(NH2)2鈫扤H3鈫�+HNCO

HNCO+H2O鈫扤H3鈫�+CO2鈫�

灏跨礌?z茅)宄ゅぅ菛鍝洨鍘濊姍閳╋攻违瀚﹀埌y(t菕ng)鑸囨按瑙ｆ硶鐩稿悓銆傚翱绱犳憾娑茬稉(j墨ng)鐢遍珮娴侀噺寰挵(hu谩n)妯″杓搁€佸埌瑷�(j矛)閲忓垎閰嶆ā濉�銆傝┎瑷�(j矛)閲忔ā濉婅兘鏍规摎(j霉)绯荤当(t菕ng)闇€姘ㄩ噺鑷嫊鎺у埗灏跨礌婧舵恫閫�(j矛n)鍏ユ祦閲�锛� 骞跺埄鐢ㄥ绺┖姘ｅ皣灏跨礌婧舵恫闇у寲骞堕€氶亷闇у寲鍣村槾鍣村叆鐔辫В鐖愬収(n猫i)锛� 鑸囩稉(j墨ng)閬庡姞鐔卞櫒鍔犵啽鍚庣殑绋€閲嬮ⅷ(f膿ng)娣峰悎鍚庡垎瑙�锛岀敓鎴怤H3銆丠2O 鍜孋O2;鍐嶉€氶亷姘ㄥ櫞灏勭郴绲�(t菕ng)鍣村叆鑴鍙嶆噳(y墨ng)鍣ㄣ€傚翱绱�?z茅)宄ら墔t闇€鎸夋(j墨)绲勯潬杩戦崑鐖愬柈鍏冨竷缃�銆傜啽瑙ｇ垚绲�(ji茅)妲�(g貌u)濡傚湒2鎵€绀恒€�


鍌崇当(t菕ng)灏跨礌?z茅)宄らェ澶筭(sh霉)涓€鑸噰鐢ㄩ浕鍔犵啽鍣ㄤ綔鐐虹█閲嬮ⅷ(f膿ng)鐨勭啽婧�锛岃┎鎶€琛�(sh霉)鍦ㄥ湅鍏�(n猫i)鎳�(y墨ng)鐢ㄨ純澶�銆傚洜闆诲姞鐔辨湰韬姛鑰楄純澶э紝灏�(d菐o)鑷村翱绱�?z茅)宄ゅ簚鍒皔(t菕ng)閬�(y霉n)琛屾垚鏈亷楂�銆傝繎骞翠締锛屾帹鍑轰簡楂樻韩?z茅)鐓旈埜Q鐔卞櫒鏇夸唬闆诲姞鐔卞櫒锛� 鍗崇敤鐓欐埃浣欑啽浣滅偤绋€閲嬮ⅷ(f膿ng)鐨勭啽婧愮殑灏跨礌?z茅)宄らェ澶筭(sh霉)锛岄檷浣庝簡灏跨礌?z茅)宄ゅ簚鍒皔(t菕ng)鐨勯亱(y霉n)琛岃不(f猫i)鐢ㄣ€傜厵姘ｆ彌鐔卞櫒涓昏鏈夌垚澶栭珮婧�?z茅)鐓旈埜Q鐔卞櫒鍜岀垚鍏�(n猫i)楂樻韩?z茅)鐓旈埜Q鐔卞櫒銆�

鐖愬楂樻韩?z茅)鐓旈埜Q鐔卞櫒鏄緸閸嬬垚楂橀亷鍚�銆侀珮鍐嶅墠鐓欓亾寮�1璺珮婧�?z茅)鐓�?鈮�800鈩�)锛屽皣涓€娆＄啽棰�(f膿ng)閫氶亷楂樻韩?z茅)鐓旈埜Q鐔卞櫒鍔犵啽鑷�450锝�600鈩�銆傝┏瑕嬪湒3銆�


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2 鎶€琛�(sh霉)缍�(j墨ng)婵�(j矛)鎬у垎鏋�

2.1 鎶€琛�(sh霉)鎬у垎鏋�

(1)灏跨礌杞�(zhu菐n)鍖栫巼銆傚翱绱犳按瑙ｇ郴绲�(t菕ng)灏跨礌杞�(zhu菐n)鍖栫巼楂樹簬灏跨礌?z茅)宄ゅ簚鍒皔(t菕ng)銆傚翱绱犳憾娑插湪姘磋В鍙嶆噳(y墨ng)鍣ㄤ腑鐧�(f膩)鐢熷彲閫嗗弽鎳�(y墨ng)锛� 灏跨礌婧舵恫鍦ㄤ竴瀹氭浠朵笅鍒嗚В鐢�(ch菐n)鐢烴H3銆丠2O鍜孋O2鐨勬贩鍚堟埃楂�銆傜敘(ch菐n)鐢熺殑娣峰悎姘ｉ珨涓嶆柗鎺掑嚭鍙嶆噳(y墨ng)鍣ㄧ敤浜庤劔纭�锛岄毃钁楀弽鎳�(y墨ng)鐨勪笉鏂烽€�(j矛n)琛�锛屽翱绱犲咕涔庡畬鍏ㄦ按瑙ｃ€傛牴鎿�(j霉)鍦嬪収(n猫i)澶氬闆诲粻灏跨礌姘磋В閬�(y霉n)琛屾暩(sh霉)鎿�(j霉)浼扮畻锛屽翱绱犳按瑙ｈ綁(zhu菐n)鍖栫巼鍙仈(d谩)99%銆�

灏跨礌?z茅)宄ゅ锠撶焊鐛�?鍊�(g猫)姘ㄥ垎瀛愬拰1鍊�(g猫)鐣版鞍閰稿垎瀛�銆傜暟姘伴吀鍦ㄧ啽瑙ｅ鐨勭挵(hu谩n)澧冩浠朵笅闆ｄ互鍒嗚В鐐烘皑姘�锛� 鐔辫В绯荤当(t菕ng)灏跨礌杞�(zhu菐n)鍖栫偤姘ㄧ殑杞�(zhu菐n)鍖栫巼鐩稿皪杓冧綆銆傜啽瑙ｇ垚瑷�(sh猫)瑷�(j矛)婧害鍦�600鈩冨乏鍙�锛� 灏跨礌婧舵恫娑叉淮鍦ㄧ啽瑙ｇ垚鍏�(n猫i)鍋滅暀鏅�(sh铆)闁撶磩鐐�7锝�8s锛� 鍏剁悊璜栬綁(zhu菐n)鍖栫巼绱勭偤90% 銆傚悓鏅�(sh铆)鏍规摎(j霉)鍦嬪収(n猫i)澶氬闆诲粻灏跨礌?z茅)宄よ喓\(y霉n)琛屾暩(sh霉)鎿�(j霉)浼扮畻锛屽翱绱�?z茅)宄ゅぅ銊濪(zhu菐n)鍖栫巼鑸囩悊璜栧€肩浉绗�銆�

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3 绺界祼(ji茅)

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